Classifying aerosol type using in situ and satellite observations over a semi-arid station, Anantapur, from southern peninsular India

Abstract

The chemical composition of aerosols is crucial for understanding aerosol radiative characteristics, classifying aerosol sources, and improving atmospheric aerosol satellite retrieval algorithms. In this study, the absorption angström exponent (AAE) and scattering angström exponent (SAE) values are derived from an aethalometer and three wavelength integrating nephelometer. MERRA-2 (Modern-Era Retrospective Study for Research and Applications) speciated aerosol optical depths and the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) aerosol subtypes are utilized for the identification of a possible aerosol type over a semi-arid station, Anantapur, in Southern peninsular India from March 2016 to February 2018. Analysis from MERRA-2 for different aerosols illustrates that sulphate aerosol optical depth (SO4 AOD) dominates (>0.16) during winter and post-monsoon, while dust aerosol optical depth (DU AOD), organic carbon optical depth (OCAOD), and sulphate aerosol optical depth (SO4 AOD) mainly contributed (>0.07) to the total AOD during summer. SO4 AOD accounted for over ∼ 50% of total AOD during winter and post-monsoon, whereas DU AOD accounted for<10% of total aerosol optical depth in the respective seasons. The seasonal mean values of SAE (AAE) were found to be 1.95 ± 0.37 (1.03 ± 0.08), 1.65 ± 0.55 (1.03 ± 0.08), 2.53 ± 0.20 (1.03 ± 0.08) and 2.66 ± 0.15 (1.03 ± 0.08) during summer, monsoon, post-monsoon, and winter, respectively. AAE and SAE classification schemes showed that during winter, summer, and post-monsoon, continental polluted aerosols dominated (>56%), while dust and marine pollution aerosols dominated (∼47%) to the total aerosols during the monsoon. Continental aerosols are predominant during all seasons except for monsoon, and result from local anthropogenic activities and the transport of mineral dust particles and smoke aerosols from the north and western India. The observed aerosol types are consistent with the air mass back-trajectory cluster analysis performed with the help of Hybrid Single-Particle Lagrangian Integrated Trajectory (HYSPLIT). The various aerosol types (absorbing and non-absorbing) and their change over a region are essential for for reducing the uncertainty in the assessment of aerosol radiative effects.