Abstract
The Raman spectra of solid HOF, DOF, and an HOF/DOF mixture have been measured. Two of the three internal vibrations (the O–F and O–H stretches) were seen, and they coincide with the bands previously found in the infrared spectrum of the solid. Six low frequency intermolecular bands found in the infrared have been interpreted in terms of a hydrogen‐bonded structure consisting of planar zigzag chains, similar to the chains that constitute the structure of solid HF.
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