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Abstract
The cyclic ketone 3-cyclopentenone has been dissociated in a molecular beam with a pulsed excimer laser to yield butadiene and CO, and the CO product state distribution has been measured using vacuum ultraviolet laser-induced fluorescence with full rovibronic state resolution. It is found that the CO rotational temperatures in =0 and 1 are 3500±140 and 7500±400 K, respectively, and that the vibrational distribution is characterized by a temperature of 1750±200 K
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