Abstract
Examination of the n→3s Rydberg transition in several methyl-substituted cyclohexanes and tetrahydropyrans (THP's) cooled in a free-jet expansion reveals the presence of two distinct molecular species. These have been assigned as pairs of conformational isomers that freeze out in the molecular beam at their room temperature populations as a result of the substantial inversion barrier of the saturated six-membered ring system
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