Charge state distributions and charge exchange cross sections of carbon in helium at 30–258 keV

Abstract

With the introduction of helium stripping in radiocarbon (14C) accelerator mass spectrometry (AMS), higher +1 charge state yields in the 200keV region and fewer beam losses are observed compared to nitrogen or argon stripping. To investigate the feasibility of even lower beam energies for 14C analyses the stripping characteristics of carbon in helium need to be further studied. Using two different AMS systems at ETH Zurich (myCADAS and MICADAS), ion beam transmissions of carbon ions for the charge states −1, +1, +2 and +3 were measured in the range of 258keV down to 30keV. The correction for beam losses and the extraction of charge state yields and charge exchange cross sections will be presented. An increase in population of the +1 charge state towards the lowest measured energies up to 75% was found as well as agreement with previous data from literature. The findings suggest that more compact radiocarbon AMS systems are possible and could provide even higher efficiency than current systems operating in the 200keV range.