Abstract
Due to their half metallic properties and high Curie temperatures Heusler alloys are potential key materials for future application in spin-based devices. One crucial aspect for device performance is the electron spin polarization at surfaces and interfaces, which in general deviates from bulk values due to the different bonding environment. Here, we present spin-resolved photoemission data on surfaces of Co2Cr1−xFexAl thin films. The influence of bulk and surface contributions on the spin-resolved spectra is discussed for x=0, x=0.4 and x=1, yielding information on disorder, surface states and calculation schemes that are consistent with our spin-resolved photoemission experiments.
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