Abstract
(1−x)(Pb0.9325La0.045)(Zr0.54Sn0.35Ti0.11)O3 (PLZST)−xPb(Mg0.5W0.5)O3 (PMW) (0≤x≤7mol%) dielectric ceramics have been investigated with regard to their phase evolution, microstructure, dielectric and energy storage properties. The PLZST modified with PMW showed a reduced sintering temperature and improved dielectric properties. According to the XRD study, a tetragonal crystal structure was found at room-temperature in the investigated range of x. The pyrochlore phase was gradually increased with increasing x. The microstructure observation revealed that the PMW doping leads to an increase in average grain size. In addition, in the composition range from 1 to 7mol%, the maximum dielectric constant increased and the Curie temperature decreased with increasing PMW concentration. From the polarization-electric field hysteresis loop measurements, higher discharged energy density and lower unreleased energy density were determined at the PMW concentration of 5mol%. The relative increase in hysteresis loss with increasing PMW concentration could be explained by the increase in interfacial polarization, as indicated by the increased pyrochlore phase.
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