Abstract
This work aims to understand the electrochemical and mechanical behaviour of silicon thin film electrodes in Lithium-ion batteries. The evolution of microstructures, mechanical stresses and material damage have been investigated via combined experimental and molecular modelling approaches. Possible mechanisms responsible for electrochemical behaviour, volume change and material failure during charging/discharging processes have been proposed. The outcome of this work will benefit the development of novel electrode materials for high-capacity Lithium-ion batteries.
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