Abstract
Quasi-random nanostructures are playing an increasingly important role in developing advanced material systems with various functionalities. Current development of functional quasi-random nanostructured material systems (NMSs) mainly follows a sequential strategy without considering the fabrication conditions in nanostructure optimization, which limits the feasibility of the optimized design for large-scale, parallel nanomanufacturing using bottom-up processes. We propose a novel design methodology for designing isotropic quasi-random NMSs that employs spectral density function (SDF) to concurrently optimize the nanostructure and design the corresponding nanomanufacturing conditions of a bottom-up process. Alternative to the well-known correlation functions for characterizing the structural correlation of NMSs, the SDF provides a convenient and informative design representation that maps processing–structure relation to enable fast explorations of optimal fabricable nanostructures and to exploit the stochastic nature of manufacturing processes. In this paper, we first introduce the SDF as a nondeterministic design representation for quasi-random NMSs, as an alternative to the two-point correlation function. Efficient reconstruction methods for quasi-random NMSs are developed for handling different morphologies, such as the channel-type and particle-type, in simulation-based microstructural design. The SDF-based computational design methodology is illustrated by the optimization of quasi-random light-trapping nanostructures in thin-film solar cells for both channel-type and particle-type NMSs. Finally, the concurrent design strategy is employed to optimize the quasi-random light-trapping structure manufactured via scalable wrinkle nanolithography process.
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