Abstract

Non-exhaust PM emissions from vehicles in real road have been conducted, but heavy vehicles have rarely been tested. In this study, PM2.5 and PM10 samples were directly collected from a tire of a moving bus and the composition was analyzed to investigate the sources of PM emissions. Driving tests were conducted at a proving ground (PG) and a city road (CR). PM2.5 emissions considerably increased when the lateral force of the tire increased and the vehicle accelerated. The PM emission rate was higher in the PG test than in the CR test because of the harsher driving conditions at PG. The emission rates of PM10 in the PG and CR tests were higher than those of PM2.5 by approximately 6 and 11 times, respectively. In the PG and CR tests, the proportions of tire wear particles (TWPs) were 4.9% and 2.1% in the PM2.5 samples, and 6.8% and 8.2% in the PM10 samples, respectively. Furthermore, TWPs with PM (TWPPM) were generated by other sources: secondary production of TWPPM by fragmentation of TWPs and resuspension of TWPPM on the road. The contributions of other sources to TWP2.5 generation were at least 6% and 57% in the PG and CR tests, respectively, whereas that to TWP10 generation was at least 3.5% in the CR test. Iron derived from brake abrasion and mineral particles was observed in the PM samples, and the Fe concentrations were higher in the PM10 samples than in the PM2.5 samples by over 9 and 18 times for the PG and CR tests, respectively. Sulfur sources, such as TWPs, exhaust gas, and bitumen, were observed in the PM samples. Based on our findings, we recommend that road wear particles should be removed from roads to reduce PM emissions upon driving.

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