Abstract
In the present study we have attempted to characterize aerosols using their optical properties over a tropical urban location of Hyderabad, India. We have analyzed three years of in-situ data on aerosol absorption from Aethalometer and scattering from Nephelometer measurements. Satellite based absorption measurements from ozone monitoring instrument, absorbing aerosol index are also analyzed to investigate the role of long range transport of dust. Further, the Cloud-Aerosol Lidar Pathfinder Satellite Observations (CALIPSO) data is used to study the vertical extent of aerosol particles as well as their sphericity using its particulate depolarization ratio. The study revealed that irrespective of seasonal variation, local anthropogenic fossil fuel aerosols form the predominant aerosol type over this site. Biomass/dust aerosols in their pure form are not present during the study period; however the spread of frequency distribution of scattering Angstrom exponent and absorption Angstrom exponent suggested their possible existence in mixed condition with local anthropogenic aerosols. The analysis of columnar aerosol absorption data during pre-monsoon period showed the dominance of UV absorbing dust aerosols in the study region. CALIPSO data analysis over study area showed that majority aerosols are confined within 2 km from the surface during winter while in pre-monsoon particles are distributed throughout the profile (~6 km) with extinction coefficient varying between 0.1-0.2 km^(-1). As the season shift from winter to pre-monsoon a change in sphericity of particle is observed. Cluster mean trajectory analysis revealed that during premonsoon majority of air mass movements (~68%) are from western side passing through dust source region like Persian Gulf and Thar Desert before entering into Indian region. During post-monsoon (~70%) and winter (~65%), majority of the air masses are coming from north-west and north-east side of the study area where biomass burning is quite frequent during this period.
Highlights
Aerosols represent unique particulate constituents that have significant impact on climate (Myhre et al, 2013)
The diurnal variation of Black Carbon (BC) is highly influenced by the diurnal evolution of atmospheric boundary layer (ABL) and its structure (Moorthy et al, 2003; Nair et al, 2007)
The mechanism for morning peak is closely associated with the fumigation effect (Nair et al, 2007), where BC in the residual layer mixes with the surface layer by mixed layer entrainment and turbulence in addition to building up of anthropogenic activities (Stull, 1998)
Summary
Aerosols represent unique particulate constituents that have significant impact on climate (Myhre et al, 2013). Satellite based absorption measurements from ozone monitoring instrument, absorbing aerosol index are analyzed to investigate the role of long range transport of dust.
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