Abstract

We have studied the morphology, structure and magnetism of Fe films thermally deposited on stepped Cu(111) by scanning tunnelling microscopy (STM), low energy electron diffraction (LEED) and magneto-optical Kerr effect (MOKE). At room temperature, in the submonolayer range Fe films grow as quasi one-dimensional stripes along the upper step edges due to a strong decoration effect. Between 1.4 and 1.8 monolayer coverage the stripes percolate and become two-dimensional films. Between 2.3 and 2.7 monolayer coverage the films undergo a structural transition from fcc(111) to bcc[110] with Kurdjumov-Sachs orientation. In the fcc range the films have a low net magnetic moment, and a perpendicular easy magnetization axis. The magnetization switches to an in-plane high-moment phase correlated with the fcc to bcc structural transformation.

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