Abstract

AbstractUsing an aerosolclimate model, we studied the temporal and spatial variations of anthropogenic PM (aerodynamic diameter 2.5 m) and coarse particulate matter (CPM; aerodynamic diameter 2.5 m) under Representative Concentration Pathway (RCP) 4.5 and RCP8.5 scenarios from 2014 to 2050. The corresponding radiative forcing and climate responses were also explored. The PM burden decreases over most continents, especially East Asia. The CPM particles increase over northern Asia, North America, and central Africa, in contrast to decrease over most regions of East Asia and North Africa. Relative to 2014, the global annual mean effective radiative forcing due to changes in PM and CPM burden are 1.17 (1.10) and 0.06 ( 0.07) W m under RCP4.5 (RCP8.5), respectively. The reduction in PM burden leads to apparent warming, especially over high latitudes of the Northern Hemisphere, with global annual mean surface air temperature increasing by 1.25 K under RCP4.5, and 1.22 K under RCP8.5. In contrast, changes in CPM result in apparent cooling over North America and northern Asia, with global annual mean changes in surface air temperature of 0.10 K for both scenarios. The Northern Hemisphere Hadley cell weakens and moves northward due to changes in PM after 2014, whereas the corresponding circulation in the Southern Hemisphere is strengthened, with the Intertropical Convergence Zone shifting to 10°N. Global annual mean precipitation increases by 0.10 mm day under both scenarios. Generally, anthropogenic PM contributes significantly to future changes in radiative forcing and climate.

Highlights

  • Atmospheric air pollutants are currently increasing sharply due to the intensification of human activities

  • Using an aerosolclimate model, we studied the temporal and spatial variations of anthropogenic PM2.5 and coarse particulate matter (CPM; aerodynamic diameter >2.5μm) under Representative Concentration Pathway (RCP) 4.5 and RCP8.5 scenarios from 2014 to 2050

  • The reduction in PM2.5 burden leads to apparent warming, especially over high latitudes of the Northern Hemisphere, with global annual mean surface air temperature increasing by 1.25 K under RCP4.5, and 1.22 K under RCP8.5

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Summary

Introduction

Atmospheric air pollutants are currently increasing sharply due to the intensification of human activities. Numerous studies have shown that can anthropogenic aerosol particles affect the environment and human health, directly changing the radiation balance of the Earth system (Bond et al, 2013; Zhang et al, 2012, 2014). They can have apparent indirect influences on the climate (Kloster et al, 2010; Zhang, 2007). The dynamic effects of long-term rising aerosol concentrations have been described as a southward shift in the Intertropical Convergence Zone (ITCZ) or changes in Hadley cells in both the Northern Hemisphere (NH) and Southern Hemisphere (SH)

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