Abstract

Catalysts are substances that assist transformation of other resourceful objects without being consumed in the process. However, the fact that their ``catalytic power'' is limited and can be depleted is often overlooked, especially in the recently developing theories on catalysis of quantum randomness utilizing building correlation with catalyst. In this work, we establish a resource theory of one-shot catalytic randomness in which uncorrelatedness is consumed in catalysis of randomness. We do so by completely characterizing bipartite unitary operators that can be used to implement catalysis of randomness using partial transpose. By doing so, we find that every catalytic channel is factorizable, and therefore there exists a unital channel that is not catalytic. We define a family of catalytic entropies that quantifies catalytically extractable R\'enyi entropies from a quantum state and show how much the degeneracy of a quantum state can boost the catalytic entropy beyond its ordinary entropy. Based on this, we demonstrate that a randomness source can be actually exhausted after a certain amount of randomness is extracted. We apply this theory to systems under superselection rules that forbids superposition of certain quantum states and find that nonmaximally mixed states can yield the maximal catalytic entropy. We discuss implications of this theory to various topics, including catalytic randomness absorption, the no-secret theorem, and the possibility of multiparty infinite catalysis.

Highlights

  • A catalyst is a substance that accelerates or initiates chemical reactions without being consumed or destroyed

  • We show that the partial transpose of a catalysis unitary operator has an operational meaning as the recovery map that recovers the input state of the catalysis encoded in the correlation with environment

  • The correlational resource theory of randomness developed in this paper is distinctly different from conventional resource theories with convex free state sets and free operations that preserve the free state set

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Summary

Introduction

A catalyst is a substance that accelerates or initiates chemical reactions without being consumed or destroyed This concept has been adopted in the context of quantum information for manipulation of entanglement, coherence, and realization of thermal operations. Even in the original context of chemistry, a catalyst C catalyzing the reaction transforming compound A into substance B may not interact with B at all even though it is not physically damaged or altered. We can interpret it as that there is a “catalytic power” that used up in catalysis, and C has no catalytic power in relation to B

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