Abstract
The catalytic oxidation of phenol over CuZSM-12 (SAR = 200) has been studied using a semi-batch slurry reactor at temperatures of 110; 120 and 130oC, and acidic neutral and basic pH. At 130oC, the phenol undergoes total conversion to carbon dioxide and water in 1.5 h. The kinetic parameters were evaluated using a modified homogeneous-heterogeneous model for the experimental data. Using this modified model, the activation energy for the catalytic oxidation process was ca. 90 kJ mol-1.
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