Abstract
The catalytic and the electrocatalytic behavior of MnOx oxides deposited on Yttria Stabilized Zirconia (YSZ) in the form of thin porous films, was studied during the reaction of methane activation at high methane to oxygen ratios. Experiments were carried out in a continuous flow well-mixed reactor (CSTR), at atmospheric total pressure and in a temperature range between 500–850 °C. It was found that the electrochemical pumping of oxygen anions (O2−) through the solid electrolyte (YSZ) affect drastically the rates of CO2, C2H4 and C2H6 formation and consequently the C2 selectivity.
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