Cascade splitting of two atomic energy levels due to multiphoton absorption

Abstract

We have theoretically and experimentally studied the spectroscopic properties of dressed levels in a strong monochromatic field, and propose a model of cascade splitting of two atomic energy levels. In this model two related dressed levels can be split into four levels, and transitions connecting four new levels will constitute spectroscopic structures. Two types of proof-in-principle experiments are performed to verify the model. One experiment measures the probe absorption spectra of a degenerate two-level atomic system with two strong monochromatic coupling fields. The system consists of ${5}^{2}{S}_{1/2},F=2$ and ${5}^{2}{P}_{3/2},{F}^{\ensuremath{'}}=3$ states of $^{87}\mathrm{Rb}$ atoms in a magneto-optical trap (MOT) as well as the cooling beams and an additional coupling field. New spectral features are observed and proven to be due to the transitions of new levels generated by splitting of the dressed levels. The other experiment measures the pump-probe spectra in a degenerate two-level atomic system with one strong monochromatic coupling field. The system consists of ${5}^{2}{S}_{1/2},F=2$ and ${5}^{2}{P}_{3/2},{F}^{\ensuremath{'}}=3$ states of the $^{87}\mathrm{Rb}$ atom in a magneto-optical trap and one coupling field. We have observed spectral features that obviously differ from the prediction that comes from the two-level dressed-atom approach. They cannot be explained by existing theories. The model of cascade splitting of two atomic energy levels is employed to explain the observations in these two types of experiments.