Abstract

The InGaN/GaN multi-quantum wells (MQWs) are prepared at the same condition by metal-organic chemical vapor deposition (MOCVD) except the thickness of cap layers additionally grown on each InGaN well layer. The photoluminescence (PL) intensity of the thin cap layer sample is much stronger than that of thicker cap layer sample. Interestingly, the thick cap layer sample has two photoluminescence peaks under high excitation power, and the PL peak energy-temperature curves show an anomalous transition from reversed V-shaped to regular S-shaped with increasing excitation power. Meanwhile, it exhibits a poorer thermal stability of thick cap layer sample under higher excitation power than that under lower excitation power. Such an untypical phenomenon is attributed to carrier redistribution between the two kinds of localized states which is induced by the inhomogeneous distribution of indium composition in thick cap layer sample. Furthermore, the luminescence of deep localized states has a better thermal stability, and the luminescence of shallow localized states has a poor thermal stability. In fact, such a severer inhomogeneous indium distribution may be caused by the degradation of subsequent epitaxial growth of InGaN/GaN MQWs region due to longer low-temperature GaN cap layer growth time.

Highlights

  • InGaN/GaN multi-quantum well (MQW) structure has received great attention due to its wide use in light-emitting diodes (LEDs) and laser diodes (LDs) [1–6]

  • Characterization To determine the average indium content, period thickness, and material quality of two InGaN/GaN MQWs, Fig. 1 The cross-sectional schematic diagram of the epilayer structures of two MQWs high-resolution x-ray diffraction (HRXRD) measurement is performed with Rigaku Ultima IV with Cu-Ka radiation (λ = 1.54 Å) that operated at 40 kV and 30 mA

  • In summary, the InGaN/GaN multi-quantum well (MQW) samples with different thickness of GaN cap layers grown on the InGaN well layers are prepared by metal-organic chemical vapor deposition system (MOCVD)

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Summary

Introduction

InGaN/GaN multi-quantum well (MQW) structure has received great attention due to its wide use in light-emitting diodes (LEDs) and laser diodes (LDs) [1–6]. It is well known that the temperaturedependent S-shaped behavior of luminescence peak energy is a fingerprint of carrier localization Many models, such as localized state ensemble (LSE) model, are proposed to. The manufactured devices like laser diodes are always operating with a higher injected carrier density [22] In this case, the photoluminescence spectra of localized states may exhibit a unique behavior at different excitation level associated with the uniformity of localized states. It is found that the thick cap layer sample shows an anomalous peak at higher energy side under high optical excitation power. This implies a co-existence of two different kinds of localized states. We can assume that the photoluminescence of deep localized states has a better thermal stability, and the photoluminescence of shallow localized states has a poor thermal stability

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