Abstract
Ferromagnetism in Mn-doped ZnO is investigated by Monte Carlo simulations assuming indirect exchange interaction via two different competing mechanisms: (i) antiferromagnetic superexchange and (ii) an oscillating carrier mediated interaction. The calculations are performed for p- and n-type samples. The Mn ion is taken as a substitutional impurity and its concentrations varied from 3% to 20%. The carrier concentrations (holes or electrons) were tested in the range of 1×1016–1×1020cm−3. These simulations showed paramagnetic, ferromagnetic, and spin-glass behaviors for the p-type samples depending on the Mn and hole concentrations. On the other hand, no phase transition was observed for the n-type samples, whatever the Mn and electron concentrations used in the simulations.
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