Carbon Dots with Blue-to-Near-Infrared Lasing for Colorful Speckle-Free Laser Imaging and Dynamical Holographic Display.

Abstract

As a new solution-processable laser material, carbon dots (CDs) offer advantages of non-toxicity, low cost, and high stability, which are conducive to the sustainable development of miniaturized lasers. We prepared full-color CDs (FC-CDs) with bright-blue, green, yellow, red, deep-red, and near-infrared (NIR) fluorescence. Their photoluminescence emission ranged from 431 to 714nm. The FC-CDs showed narrow full widths at half maximum in the range of 44-76nm, with concurrent high radiative transition rates (KR ) of 0.54-1.74 × 108 s-1 ; their performance is comparable to that of organic laser dyes, indicating their good gain potential for lasers. Laser pumping of the FC-CDs gave laser outputs at 467.3, 533.5, 577.4, 616.3, 653.5, and 705.1nm, spanning from blue to NIR region, and covering 140% of the NTSC color gamut. The FC-CDs showed high Q-factors (2000-5500), appreciable gain coefficients (9-21.5 cm-1 ), and better stability (∼100%@4-7h) than commercial laser dyes. These excellent properties make them suitable for high-quality, colorful, speckle-free laser imaging and dynamic holographic display. Our findings will be helpful in promoting the practical applications and development of solution-processable CD-based lasers. This article is protected by copyright. All rights reserved.