Abstract
The practical utilization of high energy density rechargeable lithium cells is dependent upon maintaining high capacity for the duration of the required cycle life. However, a critical, yet generic problem with room temperature lithium systems is that the capacity often declines considerably during the early stages of cycling. We report the results of our studies on electrolyte degradation which we observe after cells have undergone 300 and 700 deep cycles with 3-methylsulfolane- and 2-methyltetrahydrofuran—LiAsF 6 electrolytes, respectively.
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