Abstract

One of the major challenges to the widespread adoption of plasmonic and nano-optical devices in real-life applications is the difficulty to mass-fabricate nano-optical antennas in parallel and reproducible fashion, and the capability to precisely place nanoantennas into devices with nanometer-scale precision. In this study, we present a solution to this challenge using the state-of-the-art ultraviolet nanoimprint lithography (UV-NIL) to fabricate functional optical transformers onto the core of an optical fiber in a single step, mimicking the ‘campanile’ near-field probes. Imprinted probes were fabricated using a custom-built imprinter tool with co-axial alignment capability with sub <100 nm position accuracy, followed by a metallization step. Scanning electron micrographs confirm high imprint fidelity and precision with a thin residual layer to facilitate efficient optical coupling between the fiber and the imprinted optical transformer. The imprinted optical transformer probe was used in an actual NSOM measurement performing hyperspectral photoluminescence mapping of standard fluorescent beads. The calibration scans confirmed that imprinted probes enable sub-diffraction limited imaging with a spatial resolution consistent with the gap size. This novel nano-fabrication approach promises a low-cost, high-throughput, and reproducible manufacturing of advanced nano-optical devices.

Highlights

  • Optical transformer based near-field probes, called the “campanile”, are based on the optical transformer concept[17] that addressed most of the shortcomings of the different near-field optical probe architectures; a strong www.nature.com/scientificreports/

  • Complex photonic and plasmonic devices with high resolution have been successfully fabricated at the wafer level and shown performance comparable to those of similar devices fabricated by electron beam lithography (EBL)[26, 27]

  • We have overcome each of the challenges and developed the process to imprint an optical transformer in a single step, which has eliminated the need for any focused ion beam (FIB) milling beyond the initial step to fabricate the imprint mold

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Summary

Introduction

Optical transformer based near-field probes, called the “campanile”, are based on the optical transformer concept[17] that addressed most of the shortcomings of the different near-field optical probe architectures; a strong www.nature.com/scientificreports/. The tips can support a photon-plasmon conversion efficiency of up to 70% over a broadband wavelength range and have demonstrated sub-40 nm resolution with a normalized intensity enhancement of up to 500 times in the near infrared[20]. The fabrication of this three-dimensional nano-antennae has remained very complicated and time-consuming, requiring multiple steps of focused ion beam (FIB) milling on the tip of a tapered optical fiber. This severely limits throughput and reproducibility, and restricts the use of campanile tips to only select, priority applications in a research environment.

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