Abstract
(CH 3NH 3) 2[SnCl 6] undergoes a critical phase transition at 154.32 ± 0.06 K with the critical exponents α = 0.36 ± 0.04, α' = 0.19 ± 0.02, the critical entropy ratio 0.062 and the total transition entropy (1.60 ± 0.18) R. Infrared spectral change favors the order-disorder mechanism of the transition proposed from the thermodynamic data.
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