Calculations of strong field multiphoton processes in alkali metal atoms

Abstract

The development of a new class of laser systems, capable of producing intense radiation in the mid-infrared (MIR) regime (photon energies between 0.3 and 0.4 eV), opens the possibility of observing multiphoton processes in a new class of systems with lower ionization potentials than those previously studied. Of particular interest are the alkali metal atoms, which are true one-(valence)-electron systems. We present theoretical calculations of above threshold ionization (ATI) and high harmonic generation (HHG) from alkali metal atoms subject to 3-4 μm laser irradiation. The ATI calculations, which use a multiple gauge propagation method, show a striking dependence in the production of high-order photoelectrons on the electron-ion potential. The HHG calculations illustrate the importance of the strong ground-to-first excited state coupling in multiphoton processes in the alkali metals.