Abstract

A general theory for the calculation of interaction parameters between adsorbed species at an electrode/electrolyte-solution interface is derived and presented in a form suitable for use in conjunction with chronocoulometric studies. The theory has been applied to the adsorption of ions on a Ni single crystal, and good agreement with experimental results is obtained. It is also shown that the approximate solution to the Elovich equation can lead to considerable errors in the calculation of interaction parameters.

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