Abstract
Comparison of muon hyperfine coupling constants with the corresponding proton ones for the analogous H radical reveals considerable isotopic shifts. On isotopic substitution the bond length expectation values vary and muonic isotopic effects should be larger than with conventional isotopes such as deuterium. INDO calculations using a geometry based on MNDO-RHF calculations (with fixed CMu bond length expectation values in a Morse potential) have been carried out, giving improved values for hyperfine coupling constants and for corresponding shifts upon isotopic substitution by Mu in several radicals.
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