Abstract
The photodissociation quantum yield of chlorine in CCl 4 was determined at 308 and 337 nm using the technique of laser-induced photoacoustic calorimetry (PAC). The quantum yield for photodissociation was observed to be wavelength dependent (0.16 and 0.22 at 337 and 308 nm, respectively). This wavelength dependence originates in the excess energy that is delivered to the geminate radical pair.
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