Abstract

The reduction of the size of bubbles can improve both selectivity and conversion in gas-solid fluidized beds. Results are reported of the reduction of bubble size by the application of electric fields to uncharged, polarizable particles in fluidized beds. It is shown how average bubble diameters can be drastically reduced, with little change of the bed expansion. A literature review shows that to maintain smooth fluidization, electric fields in the direction of the gas flow, with a relatively low alternating frequency, are optimal. To measure average bubble diameters, a spectral decomposition technique of pressure fluctuation time series is used. Using this method, based on non-intrusive measurements, a characteristic length scale for bubble diameters can be found. It is shown experimentally, using video analysis, that this length scale is of constant proportionality for a given bed material and bed dimensions. The proportionality of the length scale to bubble diameter is independent of measuring height or gas velocity. With this, we have a tool for measuring bubble diameters in both 2-D and 3-D fluidized beds. Electric fields were applied to fluidized beds using thin wire electrodes placed inside the column. Both 2-D and 3-D columns were tested over a range of frequencies and field strengths. For Geldart A glass beads, an optimal range was determined at 5-20 Hz and 400-1600 V/cm fields. The reduction of bubble diameter was measured to be up to 25% for this system. Larger Geldart B glass particles show a larger reduction of bubble diameters - up to 85%. For these particles, the optimal frequency was at a higher range, 20-70 Hz. At higher frequencies (up to 100 Hz), bubble size reduction is less, but still substantial. Experiments in the 3-D column using Geldart A particles show a similar reduction in bubble diameters.

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