Abstract
A novel, 2.6-to-10-μm wavelength-tunable laser source of sub-70-fs pulses is combined with mid-IR heterodyne detection to provide a versatile laser platform for broadband two-dimensional Fourier-transform infrared spectrochronography. The mid-infrared laser output serves as both a short-pulse driver and a broadband probe for time-resolved studies of ultrafast molecular coherence, population dynamics, and multimodal energy transfer in a vast class of complex molecular systems.
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