Abstract
Linear electro-optic coefficients (r i j) of the nonlinear optical Potassium Titanyl Phosphate crystal (KTP) are calculated. Results indicate a major contribution of the short Ti-O bonds in the TiO 6 octahedra and practically an insignificant role of long Ti-O bond. Thus as far as linear electro-optic effect is concerned, the crystal behaves as if there are five bonds in the TiO 6 octahedron. The order of magnitude of the r 33 coefficient of Potassium Stannyl Phospate (KSP), the tin analogue of KTP, is estimated for which the experimental value is not known so far.
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