Abstract
Several donor-π-donor (D-π-D), acceptor-π-acceptor (A-π-A), and donor-π-acceptor (D-π-A) types of organic compounds with fluorene as π bridge and dimesitylboryl group as electron acceptor, which show strong two-photon excited blue fluorescence, have been synthesized and structurally investigated. The symmetric A-π-A type of compound exhibits the shortest wavelength of two-photon excited fluorescence (TPEF) at λ em=405 nm under the excitation of λ ex=730 nm; the unsymmetric D-π-A type of compound with diphenylamino as donor exhibits the most intense TPEF at blue region ( λ em=484 nm) with a two-photon absorption cross-section of 425 GM under λ ex=800 nm.
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