Abstract
In this paper, the progress of selective oxidation of aliphatic C–H groups with H2O2 in the presence of bioinspired manganese complexes, from 1990s until present days, is overviewed. Major milestones in catalysts development, as well as practical issues, such as efficiency, regio- and stereoselectivity, are discussed. Possible mechanism of predictably selective (non-radical) C–H oxidations over novel aminopyridine manganese complexes is considered.
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