Abstract
In recent years, visible-light photoredox catalysis has been esteemed as one sustainable and efficient catalytic strategy. The rational combination of visible-light photoredox catalysis with transition-metal catalysis and organocatalysis provides new paradigms for organic synthesis; meanwhile, this triple-synergistic catalysis enriches the synthetic scope of transition-metal catalysis and organocatalysis, with which a series of novel organic transformations have been realized. This new strategy generally enables bond constructions that would not otherwise be possible or influences the enantioselectivity or site selectivity. This perspective summarizes the recent developments of the triple-catalysis system of the combination of photocatalysis with other catalytic modes for C-C and C-X bonds forming. The opportunities and challenges faced by triple-synergistic catalysis aim to attract more momentum in aspects of updating catalytic systems, designing new reactions, and studying the mechanism in multiple catalysis.
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