Abstract
The binary interaction parameters, k ij , of 119 mixtures were determined by fitting the second cross-virial coefficients of mixtures with correlations for pure compounds [L. Meng, Y.Y. Duan, L. Li, Fluid Phase Equilib. 226 (2004) 109–120; L. Meng, Y.Y. Duan, Fluid Phase Equilib., 258 (2007) 29–33] and classical mixing rules. The mixtures included nonpolar/polar (associated), polar/polar, quantum/nonpolar (quantum) binaries. Very simple correlations for k ij of H 2O/ n-alkane, CO/nonpolar and quantum/nonpolar (quantum) binaries were successfully developed. The results show that the present correlations can accurately predict the second cross-virial coefficients.
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