Abstract

Abstract. There is a large discrepancy between the size of volcanic ash particles measured on the ground at least 500 km from their source volcano (known as cryptotephra) and those reported by satellite remote sensing (effective radius of 0.5–9 μm; 95% of particles < 17 μm diameter). Here we present new results from the fields of tephrochronology (a dating technique based on volcanic ash layers), dispersion modelling and satellite remote sensing in an attempt to understand why. A literature review and measurements of prehistoric and recent eruptions were used to characterise the size range of cryptotephra grains. Icelandic cryptotephra deposited in NW Europe has lognormal particle size distributions (PSDs) with median lengths of 20–70 μm (geometric standard deviation: 1.40–1.66; 95th percentile length: 42–126 μm). Grain-size range estimates from the literature are similar. We modelled the settling of volcanic ash using measured fall velocities of ash particles, a release height typical of moderate Icelandic eruptions (10 km), and a wind speed typical for NW Europe (10 m s−1), to show that an ash cloud can transport particles up to 80 μm diameter up to 850 km in 24 h. Thus, even moderately sized Icelandic eruptions can be expected to deposit cryptotephra on mainland Europe. Using simulated satellite infrared data for dispersion-model-derived ash clouds, we demonstrate a systematic bias towards small grain sizes in retrievals of volcanic ash clouds that contain large proportions of cryptotephra-sized grains. As the median radius of the simulated PSD increases, fewer ash-containing pixels are correctly identified. Where retrievals are made of simulated clouds with mass median radii larger than ~ 10 μm, the mean retrieved reff plateaus at around 9 μm. Assuming Mie scattering by dense spheres when interpreting satellite infrared brightness temperature difference (BTD) data puts an upper limit on retrieved particle sizes. If larger, irregularly shaped ash grains can also produce a BTD effect, this will result in further underestimation of grain size, e.g. in coarse ash clouds close to a volcano.

Highlights

  • Comparison between the fields of volcanology, dispersion modelling and satellite remote sensing reveals striking differences in published distal volcanic ash grain-size data

  • Calculations using a lognormal particle size distributions (PSDs) with geometric standard deviation (σ ) of 2.0, show that a negative brightness temperature difference (BTD) is produced for distributions with mass median radius up to 21.5 μm

  • Our results indicate that cryptotephra-sized grains should be present in distal ash clouds, while the assumption of Mie scattering by dense spheres implies that any ash cloud exhibiting a BTD is dominated by grains < 10 μm in diameter

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Summary

Introduction

Comparison between the fields of volcanology (tephrochronology), dispersion modelling and satellite remote sensing reveals striking differences in published distal volcanic ash grain-size data. Differences in their approaches and frame of reference are highlighted by the terminology of each. “coarse” ash refers to particles 1–2 mm in diameter and those < 64 μm are classified as “extremely fine” (White and Houghton, 2006); in atmospheric science airborne particles coarser than 2 μm diameter are defined as “coarse” aerosol (Seinfeld and Pandis, 2006). Volcanologists describe particle sizes via grain lengths, whereas atmospheric scientists use the particle radius. These tephra horizons are known as cryptotephra (hidden ashes) because they are found in deposits that are too thin

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