Abstract

This Article describes the effect of the excitation wavelength on the spectra of random laser emission obtained in a dye-doped polymeric system, composed of a PMMA layer and a laser dye exhibiting a bichromatic gain profile, the 3-(2,2-dicyanoethenyl)-1-phenyl-4,5-dihydro-1H-pyrazole (DCNP). We are showing that the change of pumping wavelength can be used to switch the laser emission between particular lasing bands and control the relative intensity between them if the bichromatic light amplification is achieved. We present that the random lasing phenomenon can strongly influence the resulting bichromatic emission, randomly selecting the dominating lasing band. Mentioned random band switching behavior was investigated using a statistical approach, indicating that the obtained distribution is dependent on the excitation wavelength. This feature can be used to design new types of laser-based optical random number generators that can find applications in integrated optical logic devices. To the best of the authors’ knowledge, this is the first demonstration of an optical random number generator based on the bichromatic laser dye described in the literature.

Highlights

  • This Article describes the effect of the excitation wavelength on the spectra of random laser emission obtained in a dye-doped polymeric system, composed of a PMMA layer and a laser dye exhibiting a bichromatic gain profile, the 3-(2,2dicyanoethenyl)-1-phenyl-4,5-dihydro-1H-pyrazole (DCNP)

  • We have demonstrated that luminescent dyes exhibiting gain in two separated spectral regions might be utilized as optical random number generators, if they are constituting the gain medium for random laser operation

  • The relative gain of such a system can be controlled by excitation wavelength, while random feedback is responsible for randomizing an emission process

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Summary

Introduction

This Article describes the effect of the excitation wavelength on the spectra of random laser emission obtained in a dye-doped polymeric system, composed of a PMMA layer and a laser dye exhibiting a bichromatic gain profile, the 3-(2,2dicyanoethenyl)-1-phenyl-4,5-dihydro-1H-pyrazole (DCNP). As the process of RL is highly random, the evolution of emission spectra concerning excitation wavelength change was performed in a series of 100 laser shots for the same pumping conditions.

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