Abstract
The fabrication of step-scheme (S-scheme) photocatalysts with superior redox ability for air purification is very important but remains a challenge. In this study, an S-scheme Bi12TiO20-TiO2 heterojunction is prepared for photocatalytic NO removal. The optimized Bi12TiO20-TiO2 heterojunction shows higher NO removal efficiency (42.6 %) than that of pristine Bi12TiO20 (8.7 %) and TiO2 (21.4 %) under simulated solar light irradiation. The enhanced photocatalytic activity can be attributed to the efficient separation and transfer efficiency of photoinduced electrons-hole pairs, enhanced redox ability, and increased NO adsorption capacity induced by S-scheme heterojunction between Bi12TiO20 and TiO2. The S-scheme charge transfer mechanism on Bi12TiO20-TiO2 heterojunction is proposed based on characterizations and theoretical calculations. The NO conversion process is investigated using in-situ Fourier transform infrared spectroscopy (in-situ FTIR). This study provides new insights for exploring highly efficient photocatalysts for NO removal.
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