Chemosphere | VOL. 250
Read

Beyond carbon capture towards resource recovery and utilization: fluidized-bed homogeneous granulation of calcium carbonate from captured CO2

Publication Date Jul 1, 2020

Abstract

Atmospheric carbon dioxide (CO2) imbalance due to anthropogenic emissions has direct impact in climate change. Recent advancements in the mitigation of industrial CO2 emissions have been brought about by a paradigm shift from mere CO2 capture onto various adsorbents to CO2 conversion into high value products. The present study proposes a system which involves the conversion of CO2 into high purity, low moisture, compact and large CaCO3 solids through homogeneous granulation in a fluidized-bed reactor (FBR). In the present study, synthetic solutions of potassium carbonate (K2CO3) and calcium hydroxide (Ca(OH)2) were used as sources of carbonate and precipitant, respectively. The effects of the degree of supersaturation (S) as chemical loading and influx flow rate (QT) as hydraulic loading on CaCO3 granulation efficiency were investigated. In the study, S was varied from 10.2 to 10.8 and QT from 40 to 80mLmin-1 while the operating pH and calcium-is-to-carbonate molar ratio ([Ca2+]/[CO32-]) were set at 10±0.2 and 1.50, respectively. Results showed that carbonate ions end product distribution had a highest carbonate granulation efficiency at [Carbonate]G of 95-96% using S of 10.6 and QT of 60mLmin-1. Characterization of the granules confirmed high purity calcium carbonate. Overall, the transformation of industrial CO2 emissions into a valuable solid product can be a significant move towards the mitigation of climate change from anthropogenic emissions.

Concepts
Powered ByUnsilo

Homogeneous Granulation
Mitigation Of Climate Change
Impact In Climate Change
High Value Products
Atmospheric Carbon Dioxide
Chemical Loading
Solutions Of Calcium Hydroxide
Hydraulic Loading
Carbon Capture
Industrial Emissions

Introducing Weekly Round-ups!Beta

Powered by R DiscoveryR Discovery

Round-ups are the summaries of handpicked papers around trending topics published every week. These would enable you to scan through a collection of papers and decide if the paper is relevant to you before actually investing time into reading it.

Climate change Research Articles published between Aug 08, 2022 to Aug 14, 2022

R DiscoveryAug 15, 2022
R DiscoveryArticles Included:  5

Introduction: There is no consensus on the policies that should be seen as implicitly pricing carbon (see World Bank (2019a) for a discussion). The OE...

Read More

Gender Equality Research Articles published between Aug 08, 2022 to Aug 14, 2022

R DiscoveryAug 15, 2022
R DiscoveryArticles Included:  4

I would like to thank Anna Khakee, Federica Zardo and Ragnar Weilandt for their very useful comments as well as the participants of the workshop of 21...

Read More

Coronavirus Pandemic

You can also read COVID related content on R COVID-19

R ProductsCOVID-19

ONE PROBLEM . ONE PURPOSE . ONE PLACE

Creating the world’s largest AI-driven & human-curated collection of research, news, expert recommendations and educational resources on COVID-19

COVID-19 Dashboard

Disclaimer: All third-party content on this website/platform is and will remain the property of their respective owners and is provided on “as is” basis without any warranties, express or implied. Use of third-party content does not indicate any affiliation, sponsorship with or endorsement by them. Any references to third-party content is to identify the corresponding services and shall be considered fair use under The Copyright Law.