Abstract
The impacts of sintered titanium powder diameter and porous transport layer (PTL) porosity on reactant transport and PTL-catalyst layer (CL) contact in the polymer electrolyte membrane (PEM) electrolyzer were studied using stochastic generation and a pore network model. Enhanced reactant transport was established with increased powder diameter and porosity, observed through increases in single- and two-phase permeabilities. Compared to increasing the powder diameter, increasing the PTL porosity dominated increases in permeabilities, especially at higher porosities (e > 40%). However, we observed a trade-off whereby increasing the powder diameter led to increased surface roughness at the PTL-CL interface. High roughnesses were observed at porosities > 40%. In conclusion, the powder diameter and porosity must be strategically selected for the desired target operating conditions of the PEM electrolyzer.
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