Abstract
The effect of precursor vapor pressure on LiNbO 3 and LiTaO 3 film stoichiometry is compared for single and double alkoxides. Stoichiometric evaporation can be achieved in an appropriate temperature and pressure range according to the precursor sublimate composition analysis. The deposited LiTaO 3 films from LiTa(l-OC 4H 9) 6 were stoichiometric and epitaxial when a lattice-matched single-crystal substrate was used. The stoichiometry of the film was assessed by Rutherford backscattering and precision lattice parameter measurements. The high quality of the epitaxial layer was confirmed by high-resolution double- and triple-axes X-ray diffraction.
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