Abstract
In order to elucidate state-to-state dissociation dynamics of inner-shell photoexcited molecules, we have investigated ionic fragmentations by energy-resolved Auger-electron-photoion coincidence techniques. Results are presented for the fragmentation of SiF 4 following the Si 2p photoionization. It is found that the fragmentation patterns strongly depend on the Auger final states. The dissociation pathways are discussed on the basis of comparison between the present results and the appearance potential of the ionic species and ion pairs in the literature.
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