Abstract

Measurements of quantum correlations are reported for a frequency difference of 25 THz between the signal and idler output fields generated by a subthreshold nondegenerate optical parametric oscillator. By simultaneously exciting a two-photon transition in atomic Cs by a combination of signal, idler, and ``references oscillator'' fields, we record modulation of the excited-state population due to quantum interference between two alternative excitation pathways. The observed phase-sensitive modulation is proportional to the correlation function 〈E-|${\mathrm{Ax}}_{\mathrm{s}}$E-|${\mathrm{Ax}}_{\mathrm{i}}$〉 for the quantized signal and idler fields.

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