Atomic structure study of the pyrochloreYb2Ti2O7and its relationship with low-temperature magnetic order

Abstract

Exchange interactions with itinerant electrons are known to act as a relaxation mechanism for individual local spins. The same exchange interactions are also known to induce the so called RKKY indirect exchange interaction between two otherwise decoupled local spins. Here we show that both the spin relaxation and the RKKY coupling can be seen as the dissipative and reactive response to the coupling of the local spins with the itinerant electrons. We thereby predict that the spin relaxation rates of magnetic nanostructures of exchanged coupled local spins, such as as nanoengineered spin chains, have an oscillatory dependence on $k_F d$ , where $k_F$ is the Fermi wave length and $d$ is the inter-spin distance, very much like the celebrated oscillations in the RKKY interaction. We demonstrate that both $T_1$ and $T_2$ can be enhanced or suppressed, compared to the single spin limit, depending on the interplay between the Fermi surface and the nanostructure geometrical arrangement. Our results open a route to engineer spin relaxation and decoherence in atomically designed spin structures.