Abstract

The absorption of traveling photons resonant with electric dipole transitions of an atomic gas naturally leads to electric dipole spin wave excitations. For a number of applications, it would be highly desirable to shape and coherently control the spatial waveform of the spin waves before spontaneous emission can occur. This paper details a recently developed optical control technique to achieve this goal, where counter-propagating, shaped sub-nanosecond pulses impart sub-wavelength geometric phases to the spin waves by cyclically driving an auxiliary transition. In particular, we apply this technique to reversibly shift the wave vector of a spin wave on the $D2$ line of laser-cooled $^{87}$Rb atoms, by driving an auxiliary $D1$ transition with shape-optimized pulses, so as to shut off and recall superradiance on demand. We investigate a spin-dependent momentum transfer during the spin-wave control process, which leads to a transient optical force as large as $\sim 1\hbar k$/ns, and study the limitations to the achieved $70\sim 75\%$ spin wave control efficiency by jointly characterizing the spin-wave control and matterwave acceleration. Aided by numerical modeling, we project potential future improvements of the control fidelity to the $99\%$ level when the atomic states are better prepared and by equipping a faster and more powerful pulse shaper. Our technique also enables a background-free measurement of the superradiant emission to unveil the precise scaling of the emission intensity and decay rate with optical depth.

Highlights

  • Spontaneous emission is typically a decoherence effect to avoid when levels in small quantum systems are chosen to encode information for, e.g., quantum computation, simulation, or sensing [1,2,3,4]

  • Instead of using ultrafast lasers, here we develop a wide-band pulse-shaping technique based on fiber-based sideband electro-optical modulation of a cw laser [30], with up to 13 GHz modulation bandwidth, to support the flexibly programmable error-resilient spin wave control

  • Compared with previous work on spectroscopy based upon perturbative nonlinear optical effects [41,42,43], our technique is unique in that we steer the atomic state over the entire Bloch sphere of the two-level system to achieve the geometric robustness toward perfect spin-wave control set by Eq (2)

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Summary

INTRODUCTION

Spontaneous emission is typically a decoherence effect to avoid when levels in small quantum systems are chosen to encode information for, e.g., quantum computation, simulation, or sensing [1,2,3,4]. What is needed is a technique to efficiently and coherently alter the phase-matching condition of collective atomic excitations in the temporal domain—that is, to modify the wave vector of the spin waves and coherently convert between superradiant and subradiant modes—on rapid timescales faster than the typical emission time of atoms themselves. We exploit the ability to shift the dipole spin-wave vector to measure phase-matched forward collective emission in a background-free manner. To ensure completeness and to provide better context, key ideas from Ref. [30] are repeated in this paper

Preparation and control of optical spin waves
Error-resilient spin-wave control
Dynamics of controlled emission
EXPERIMENTAL RESULTS
Intensity and decay of the redirected emission
Reversible shift of spin-wave k vector
Optical acceleration
Control efficiency: calibration and optimization
DISCUSSIONS
Toward perfect control with pulse shaping
Summary and outlook
Resonant OD and atom number measurements
Collective spontaneous emission from a dilute gas of two-level atoms
Simulation of spin-wave dynamics supported by noninteracting atoms
Reconstructing the controlled spin-wave dynamics
Consistent recall at selected t3 delay

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