Abstract
Abstract Clouds and aerosols have a large, yet highly uncertain, effect on changes in Earth’s climate. A factor of particular note is the role played by ice-nucleating particles, which remains poorly understood. The mineral K-feldspar (Kfs) has recently been shown by a number of independent studies to nucleate ice in mixed-phase cloud conditions far more efficiently than other common minerals. Here, global atmospheric Kfs flux through geologic time is estimated; constrained by records of secular continental crust and biosphere evolution, plate tectonics, volcanism, glaciation, and attendant trends in land surface stability. The analysis reveals that Kfs flux today is at neither extreme of the range estimated across geological time. The present-day Kfs flux, however, is likely to be among the most spatially and temporally variable due to land surface change. The concept of an ice-nucleation efficiency factor that can be calculated from rocks, and also eolian sediments and soils, is proposed. This allows the impact of paleo-atmospheric dust to be estimated through the rock record alongside meteorological and atmospheric composition considerations. With the reasonable assumption that the ice-nucleating properties of Kfs are themselves independent of the background climate state, a better understanding of Kfs flux across a range of spatial and temporal scales will advance understanding of climate processes and interactions.
Highlights
Mineral particles that act as ice-nucleating particles (INPs; see Vali et al, 2005) are volumetrically rare, yet they exert an important influence upon the microphysics of clouds (Hoose and Möhler, 2012; Nenes et al, 2014; Murray et al 2012) and radiative forcing of climate and precipitation (DeMott et al, 2010; Storelvmo et al, 2011)
This study aims to provide a better understanding of Kfs availability and, by extension, possible flux to the atmosphere from deep time to the present, in order to inform our view of the role of Kfs and its impact as an INP through time
As the corollary of Felsic large igneous provinces (F-LIPs) spikes, dips may be caused by extensive cover of continental flood basalt by mafic LIPs, estimation of lateral extent is difficult to assess in the Precambrian (Ernst and Buchan, 2001)
Summary
Mineral particles that act as ice-nucleating particles (INPs; see Vali et al, 2005) are volumetrically rare, yet they exert an important influence upon the microphysics of clouds (Hoose and Möhler, 2012; Nenes et al, 2014; Murray et al 2012) and radiative forcing of climate and precipitation (DeMott et al, 2010; Storelvmo et al, 2011) These mineral aerosols may account for a large proportion of the INPs present within mixed-phase clouds below ~-15 °C on Earth (Atkinson et al, 2013). This study aims to provide a better understanding of Kfs availability and, by extension, possible flux to the atmosphere from deep time to the present, in order to inform our view of the role of Kfs and its impact as an INP through time
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