Abstract
Asymmetric light reflectance associated with localized surface plasmons excited in metal nanoparticles on a quartz substrate is observed and analyzed. This phenomenon is explained by the superposition of two waves, the wave reflected by the air/quartz interface and that reflected by the metal nanoparticles, and the resulting interference effects. Far field behavior investigation suggests that zero reflection can be achieved by optimizing the density of metal nanoparticles. Near field behavior investigation suggests that the coupling efficiency of localized surface plasmon can be additionally enhanced by separating the metal NPs from substrates using a thin film with refractive index smaller than the substrate. The latter behavior is confirmed via surface-enhanced Raman spectroscopy studies using metal nanoparticles on Si/SiO2 substrates.
Highlights
By including a thin film with optimized thickness
To a certain degree, this phenomenon is similar to the asymmetric light reflectance effect we have reported previously in AAO on glass[27]
We observed the asymmetric light reflectance phenomenon in metallic NPs fabricated on quartz substrate
Summary
By including a thin film with optimized thickness. This behaviour provides a general method to enhance the LSPs coupling efficiency that may improve the performance of the LSPs based devices for a variety of applications. For the sample consisting of Ag NPs on quartz substrate, peaks are seen in the reflectance spectra when light is incident from both sides.
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