Abstract

Abstract. Clear-sky, direct shortwave aerosol radiative forcing (ARF) has been estimated over the Indian region, for the first time employing multi-year (2009–2013) gridded, assimilated aerosol products, as an important part of the South West Asian Aerosol Monsoon Interactions (SWAAMI) which is a joint Indo-UK research field campaign focused at understanding the variabilities in atmospheric aerosols and their interactions with the Indian summer monsoon. The aerosol datasets have been constructed following statistical assimilation of concurrent data from a dense network of ground-based observatories and multi-satellite products, as described in Part 1 of this two-part paper. The ARF, thus estimated, is assessed for its superiority or otherwise over other ARF estimates based on satellite-retrieved aerosol products, over the Indian region, by comparing the radiative fluxes (upward) at the top of the atmosphere (TOA) estimated using assimilated and satellite products with spatiotemporally matched radiative flux values provided by CERES (Clouds and Earth's Radiant Energy System) single-scan footprint (SSF) product. This clearly demonstrated improved accuracy of the forcing estimates using the assimilated vis-à-vis satellite-based aerosol datasets at regional, subregional and seasonal scales. The regional distribution of diurnally averaged ARF estimates has revealed (a) significant differences from similar estimates made using currently available satellite data, not only in terms of magnitude but also the sign of TOA forcing; (b) the largest magnitudes of surface cooling and atmospheric warming over the Indo-Gangetic Plain (IGP) and arid regions from north-western India; and (c) negative TOA forcing over most parts of the Indian region, except for three subregions – the IGP, north-western India and eastern parts of peninsular India where the TOA forcing changes to positive during pre-monsoon season. Aerosol-induced atmospheric warming rates, estimated using the assimilated data, demonstrate substantial spatial heterogeneities (∼0.2 to 2.0 K d−1) over the study domain with the IGP demonstrating relatively stronger atmospheric heating rates (∼0.6 to 2.0 K d−1). There exists a strong seasonality as well, with atmospheric warming being highest during pre-monsoon and lowest during winter seasons. It is to be noted that the present ARF estimates demonstrate substantially smaller uncertainties than their satellite counterparts, which is a natural consequence of reduced uncertainties in assimilated vis-à-vis satellite aerosol properties. The results demonstrate the potential application of the assimilated datasets and ARF estimates for improving accuracies of climate impact assessments at regional and subregional scales.

Highlights

  • The uncertainties in aerosol radiative forcing (ARF) pose primary challenges in the assessment of climatic implications of atmospheric aerosols at global, regional and even subregional scales (Schwartz, 2004; Boucher et al, 2013)

  • As the dARF calculation has to account for the signs of the respective ARF estimates, positive dARFTOA indicates smaller magnitudes of AS ARFTOA visà-vis SR ARFTOA, and vice versa when both RF estimates are negative, which is the case in general

  • Clear-sky direct aerosol radiative forcing over the Indian region by incorporating gridded, assimilated, multi-year (2009–2013) datasets for monthly aerosol optical depth (AOD) and single scattering albedo (SSA) in Santa Barbara DIScrete Ordinate Radiative Transfer (DISORT) Atmospheric Radiative Transfer (SBDART) and compared its spatiotemporal features with those in ARF estimated using presently available satellite-retrieved aerosol products

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Summary

Introduction

The uncertainties in aerosol radiative forcing (ARF) pose primary challenges in the assessment of climatic implications of atmospheric aerosols at global, regional and even subregional scales (Schwartz, 2004; Boucher et al, 2013). There have been several estimates of global ARF by employing general circulation models (GCMs) or chemistry transport models (CTMs) making use of aerosol emission inventories (Jacobson, 2001; Takemura et al, 2002; Myhre et al, 2007, 2009; Kim et al, 2008) These studies have highlighted the regional and temporal heterogeneity in aerosol forcing, but the actual forcing values reported have significant uncertainties emanating mainly from those in the input inventories, meteorology and assumptions made in aerosol– chemistry processing. The primary findings of the present work are summarized

Database
ARF estimation
Spatial distribution of aerosol radiative forcing
Comparison with CERES measurements
Atmospheric heating rate estimation
Seasonal and subregional features
IGP 2 NE 3 PI 4 WAR
Summary
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