Assessment of radioactivity in particulate matter and soil from selected mining towns of Erongo region, Namibia

Abstract

The presence of radionuclides in particulate matter (PM) associated with mining operations in communities located at the edge of the mine sites have been either greatly ignored or poorly understood, leading to the underestimations of the radionuclides concentrations in PM and health impact. In this study, measurements of radioactivity in PM and soil were made in the two mining towns of Karibib and Arandis to assess the human health radiological impact on the people around the mining sites. Dust fall samples were collected for a period of six months i.e. May 2017 to October 2017 using open bucket sampler procedure according to the American Society for Testing and Materials Standard Method (ASTM D1739) while some soil samples were collected using a soil auger. The samples were measured for the presence radionuclides using a well calibrated gamma-ray spectrometer coupled with a high purity germanium detector.In particulate matter samples, the mean activity concentrations of 226Ra, 238U, 232Th, 210Pb, and 40K were found to be 81.24±1.00, 57.99±2.61, 72.10±1.67, 55.89±6.21, 682±19.81 Bq.kg−1, respectively. Similarly, in soil samples, the mean activity concentrations were found to be 66.41±1.77 Bq.kg−1 for 226Ra, 52.79±3.40 Bq.kg−1 for 238U, 71.30±2.40 Bq.kg−1 for 232Th, Bq.kg−1 for 71.50±5.99 210Pb and 797.36±18.26 Bq.kg−1 for 40K. The activity concentrations revealed higher levels of radionuclides associated with the 238U series, which were distributed unevenly across the sites. The results were comparable to global values of 11 to 64 Bq.kg−1 for 238U, 17 to 60 Bq.kg−1 for 232Th, and 140 to 850 Bq.kg−1 for 40K.The activity concentrations were used to compute the absorbed dose (D), annual effective dose equivalent (AEDE), radium equivalent activity concentrations (Ra eq), external and internal hazard indices (H ex and H in), Gamma Index (Iγ), Alpha Index (Iα) and excess lifetime cancer risk (ELCR). The mean radiological parameters in most samples were found to be within acceptable limits, with Raeq 370 Bq.kg−1, which corresponds to an upper safe limit of AEDE of 1 mSv.yr−1, the prescribed safe limit by the International Commission on Radiological Protection (ICRP), and thus the potential radiological health effects may not be significant.