Assessment of Black Carbon, optical properties and aerosol radiative forcing at Pranmati basin Himalayan critical zone observatory

Abstract

The study aimed to understand the optical properties of Black Carbon (BC) and radiative forcing over a data deficient Himalayan region focusing on critical zone observatory employing ground-based measurements by Aethalometer for BC and satellite retrieval techniques for optical properties during mid-May-June 2022 and January–May 2023.BC mass concentration ranged from 0.18 to 4.43 μgm−3, exhibit a mean of 1.47 ± 0.83 μgm−3 with higher summer concentration (1.51 ± 0.94 μgm−3) than winter (1.39 ± 0.61 μgm−3). The average Absorption Ångström Exponent observed to be significantly higher than unity (1.77 ± 0.31) over the studied high-altitude Himalayan region, suggesting the dominance of biomass-burning aerosol. Higher aethalometer derived compensation parameter (K) in winter suggesting locally originated BC while, lower K value in summer suggesting aged BC transported from Indo-Gangetic Plains.Optical properties calculated from “Optical Properties of Aerosol and Cloud” (OPAC) model are used in the “Santa Barbara DISORT Atmospheric Radiative Transfer” (SBDART) model to calculate the aerosol Direct Radiative Force (DRF). The entire studied period is characterized by the predominance of absorbing aerosols, particularly BC, increasing Aerosol Optical Depth, Asymmetric Parameters and decreasing Single Scattering Albedo, leading to a considerable increase in atmospheric radiative forcing (+0.9 Wm−2, top of atmosphere) and Heating Rate (0.36 KDay−1). The mean radiative forcing within atmosphere during summer was higher (+14.29 Wm−2) relative to the winter (+12.00 Wm−2), emphasizing the impact of absorbing aerosols on regional warming and potential glacier melting in the Himalayas at a faster rate. Urgent policy consideration for the reduction of absorbing aerosols is highlighted, recognizing the critical roles of Black Carbon in the changing behaviour of Critical Zone observatory. The study's data serve as a valuable resource to understanding and addressing uncertainties in climate models, aiding effective policy implementation for Black Carbon reduction.