Assessing the accumulation of sorbed isotope 137Cs within the upper components of the fluvial network in the zone of Chernobyl contamination

Abstract

We examine the use of two alternative techniques for assessing the redistribution volumes of sorbed 137Cs within the upper components of the fluvial network, based on the concept of catchment as a lithodynamical system. In terms of one of them, we made a substantive analysis of changes in reserves on accumulative positions where the 137Cs distribution curves showed a significant increase in radionuclide content levels. We carried out a typization o the accumulation surfaces in order to extrapolate data, obtained for a group of soil profiles, to the territory of the entire catchment and to make a direct assessment of the increases in accumulation. An alternative technique was used to assess the volumes of accumulated sediment loads on accumulative positions by analyzing the 137Cs distribution curves, and to correlate with denudation zones in the drainage area under consideration. Values of the wash-out rates for the period 1986–2012 have been obtained, which are necessary for the formation of the accumulative layer observed. We calculated the volume of 137Cs swept away during 26 years after the Chernobyl accident, based on information regarding the volumes of initial reserves in the denudation zones and a correlation between the erosion rate and a specific reduction in reserves. It is established that the technique on the basis of analyzing the wash-out zones featuring high economical efficiency can be used in assessing 137Cs migration for larger territories with relatively low labor-consuming effort.